Why is Control-C ambiguous? Oh wait, you guys use Control-C for copy, but you have forgotten that both Windows and Linux support Control-Insert for copy. That's what I use.
Not using the combination for one of its ambiguous purposes does not strip it of ambiguity, you've just trained yourself to avoid those circumstances.
That, of course, is one of the pain points that the article addresses: Training yourself to do so is additional cognitive load that never should have been necessary in the first place.
I flip between macOS and Linux and, occasionally, Windows. On one of my laptops, insert is also a Fn switch away, so I have to either remember that this machine needs Ctrl-Fn-F11 specifically when I'm copying from terminal.
On another keyboard I have the same problem, but insert is mapped to a different key entirely, so it is ctrl-fn-equals, and fn is on the opposite side of the keyboard from ctrl.
Contort my fingers in which way on which keyboard? Mental load and annoyance I don't need.
That would not be a good approach on Macs where most users are using reduced/laptop keyboards that have no Insert key.
In this respect, Apple got pretty lucky. Most users were not using reduced keyboards in 1987 when they originally decided to add the Control key separate from Command. Plus, Mac OS didn't even have a native terminal at the time; I assume there were terminal emulators for networking/serial use but I can't imagine that was top-of-mind for Apple either.
Regardless, Cmd-C is definitely a more convenient shortcut than Control-Insert, even if you do have the keys for the latter.