I investigated a gradient-descent-based concept adjacent to this back in like 2023 [0] inspired by the original 3DGS paper, I was pretty happy with the results I got with back-to-front alpha-blending and polar-coordinate gaussians for variable-curvature brush strokes. One of these days I should add another example gif to the repo besides just the Mona Lisa one that's currently there, but that's the only one I've got at the moment unfortunately.
Neat, watching it paint as an animation is pretty fun.