I recently read 'Maniac' by Benjamin Labatut, which also tracks the life of Johnny von Neumann. It is a wonderful read - very eloquently put together, giving accounts of the man from the perspectives of several people in his life.
Not only does it capture the alien-like genius of the protagonist, but also described his particular emotional and social character in a way that I have not seen written elsewhere. Highly recommended.
I looked at the description and this part: "Braiding fact with fiction, Benjamín Labatut takes us on a journey to the frontiers of rational thought" - gave me pause. The Braiding fact with fiction part. Are there clear demarcations between fact and fiction?
Seconding this. Maniac is a beautifully written book about von Neumann. It also led me to Benjamin Labatut's When We Cease to Understand the World, another great read.